One time I saw GM Gawain Jones playing a blitz game where he castled by placing one hand on his King and Rook. With a quick twist, the pieces were in the castled position. It happened so quickly, I didn't quite see how he did it, but I was mighty impressed.
Normally, a player will move his King, then use the same hand to move the Rook afterwards, but has anybody else seen (or done themselves) a one-motion castling?